League of Legends updated their lobby and now runs on a web-based client. Web-based content cannot be captured using Game Capture.

As a workaround, you can go on Add Source > Desktop Capture > Apps and select the lobby window and add the League of Legends in-game window as Game Capture on top of it.

XBC Source list showing one source for LOL's game screen (game capture) and a window capture source for LOL's client process

This way, you’ll be able to record or stream the game lobby and automatically switch to the main game when you start playing.
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